Abstract

The collective oscillation of electrons located in the conduction band of metal nanostructures being still energized, with the energy up to the bulk plasmon frequency, are called nonequilibrium hot electrons. It can lead to the state-filling effect in the energy band of the neighboring semiconductor. Here, we report on the incandescent-type light source composed of Au nanorods decorated with single Ga-doped ZnO microwire (AuNRs@ZnO:Ga MW). Benefiting from Au nanorods with controlled aspect ratio, wavelength-tunable incandescent-type lighting was achieved, with the dominating emission peaks tuning from visible to near-infrared spectral regions. The intrinsic mechanism was found that tunable nonequilibrium distribution of hot electrons in ZnO:Ga MW, injected from Au nanorods, can be responsible for the tuning emission features. Apart from the modification over the composition, bandgap engineering, doping level, etc., the realization of electrically driving the generation and injection of nonequilibrium hot electrons from single ZnO:Ga MW with Au nanostructure coating may provide a promising platform to construct electronics and optoelectronics devices, such as electric spasers and hot-carrier-induced tunneling diodes.

© 2019 Chinese Laser Press

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2019 (10)

S. Kahmann and M. A. Loi, “Plexcitonics — fundamental principles and optoelectronic applications,” J. Mater. Chem. C 7, 1821–1853 (2019).
[Crossref]

R.-J. Shiue, Y. Gao, C. Tan, C. Peng, J. Zheng, D. K. Efetov, Y. D. Kim, J. Hone, and D. Englund, “Thermal radiation control from hot graphene electrons coupled to a photonic crystal nanocavity,” Nat. Commun. 10, 109 (2019).
[Crossref]

M. Jiang, W. Mao, X. Zhou, C. Kan, and D. Shi, “Wavelength-tunable waveguide emissions from electrically driven single ZnO/ZnO:Ga superlattice microwires,” ACS Appl. Mater. Interfaces 11, 11800–11811 (2019).
[Crossref]

Z. Zhang, Y. Ning, and X. Fang, “From nanofibers to ordered ZnO/NiO heterojunction arrays for self-powered and transparent UV photodetectors,” J. Mater. Chem. C 7, 223–229 (2019).
[Crossref]

H. Shan, Y. Yu, X. Wang, Y. Luo, S. Zu, B. Du, T. Han, B. Li, Y. Li, J. Wu, F. Lin, K. Shi, B. K. Tay, Z. Liu, X. Zhu, and Z. Fang, “Direct observation of ultrafast plasmonic hot electron transfer in the strong coupling regime,” Light Sci. Appl. 8, 9 (2019).
[Crossref]

Z. Yang, K. Du, F. Lu, Y. Pang, S. Hua, X. Gan, W. Zhang, S. J. Chua, and T. Mei, “Silica nanocone array as a template for fabricating a plasmon induced hot electron photodetector,” Photon. Res. 7, 294–299 (2019).
[Crossref]

Y. Ni, C. Kan, L. He, X. Zhu, M. Jiang, and D. Shi, “Alloyed Au-Ag nanorods with desired plasmonic properties and stability in harsh environments,” Photon. Res. 7, 558–565 (2019).
[Crossref]

B. Huang, Z. Kang, J. Li, M. Liu, P. Tang, L. Miao, C. Zhao, G. Qin, W. Qin, S. Wen, and P. N. Prasad, “Broadband mid-infrared nonlinear optical modulator enabled by gold nanorods: towards the mid-infrared regime,” Photon. Res. 7, 699–704 (2019).
[Crossref]

W. Xu, Y. Shi, F. Ren, D. Zhou, L. Su, Q. Liu, L. Cheng, J. Ye, D. Chen, R. Zhang, Y. Zheng, and H. Lu, “Magnesium ion-implantation-based gallium nitride p-i-n photodiode for visible-blind ultraviolet detection,” Photon. Res. 7, B48–B54 (2019).
[Crossref]

S. Kahmann and M. A. Loi, “Hot carrier solar cells and the potential of perovskites for breaking the Shockley–Queisser limit,” J. Mater. Chem. C 7, 2471–2486 (2019).
[Crossref]

2018 (20)

T. A. Growden, W. Zhang, E. R. Brown, D. F. Storm, D. J. Meyer, and P. R. Berger, “Near-UV electroluminescence in unipolar-doped, bipolar-tunneling GaN/AlN heterostructures,” Light. Sci. Appl. 7, 17150 (2018).
[Crossref]

P. Wang, A. V. Krasavin, M. E. Nasir, W. Dickson, and A. V. Zayats, “Reactive tunnel junctions in electrically driven plasmonic nanorod metamaterials,” Nat. Nanotechnol. 13, 159–164 (2018).
[Crossref]

I. F. Teixeira, E. C. M. Barbosa, S. C. E. Tsang, and P. H. C. Camargo, “Carbon nitrides and metal nanoparticles: from controlled synthesis to design principles for improved photocatalysis,” Chem. Soc. Rev. 47, 7783–7817 (2018).
[Crossref]

K. Zhang, Y. Liu, J. Zhao, and B. Liu, “Nanoscale tracking plasmon-driven photocatalysis in individual nanojunctions by vibrational spectroscopy,” Nanoscale 10, 21742–21747 (2018).
[Crossref]

C. Karnetzky, P. Zimmermann, C. Trummer, C. D. Sierra, W. Martin, R. Kienberger, and A. Holleitner, “Towards femtosecond on-chip electronics based on plasmonic hot electron nano-emitters,” Nat. Commun. 9, 2471 (2018).
[Crossref]

T. Heilpern, M. Manjare, A. O. Govorov, G. P. Wiederrecht, S. K. Gray, and H. Harutyunyan, “Determination of hot carrier energy distributions from inversion of ultrafast pump-probe reflectivity measurements,” Nat. Commun. 9, 1853 (2018).
[Crossref]

C. De Melo, M. Jullien, Y. Battie, A. En Naciri, J. Ghanbaja, F. Montaigne, J. F. Pierson, F. Rigoni, N. Almqvist, A. Vomiero, S. Migot, F. Mucklich, and D. Horwat, “Tunable localized surface plasmon resonance and broadband visible photoresponse of Cu nanoparticles/ZnO surfaces,” ACS Appl. Mater. Interfaces 10, 40958–40965 (2018).
[Crossref]

S. Liu, M.-Y. Li, D. Su, M. Yu, H. Kan, H. Liu, X. Wang, and S. Jiang, “Broadband high sensitivity ZnO colloidal quantum dots/self-assembled Au nanoantennas heterostructures photodetectors,” ACS Appl. Mater. Interfaces 10, 32516–32525 (2018).
[Crossref]

Y. Ning, Z. Zhang, F. Teng, and X. Fang, “Novel transparent and self-powered UV photodetector based on crossed ZnO nanofiber array homojunction,” Small 14, 1703754 (2018).
[Crossref]

C.-C. Hou, H.-M. Chen, J.-C. Zhang, N. Zhuo, Y.-Q. Huang, R. A. Hogg, D. T. Childs, J.-Q. Ning, Z.-G. Wang, F.-Q. Liu, and Z.-Y. Zhang, “Near-infrared and mid-infrared semiconductor broadband light emitters,” Light Sci. Appl. 7, 17170 (2018).
[Crossref]

Y. Y. Cai, J. G. Liu, L. J. Tauzin, D. Huang, E. Sung, H. Zhang, A. Joplin, W. S. Chang, P. Nordlander, and S. Link, “Photoluminescence of gold nanorods: Purcell effect enhanced emission from hot carriers,” ACS Nano 12, 976–985 (2018).
[Crossref]

G. Wei, B. Xu, and H. L. Dai, “Super bright luminescent metallic nanoparticles,” J. Phys. Chem. Lett. 9, 4155–4159 (2018).
[Crossref]

S. K. Cushing, C. J. Chen, C. L. Dong, X. T. Kong, A. O. Govorov, R. S. Liu, and N. Wu, “Tunable nonthermal distribution of hot electrons in a semiconductor injected from a plasmonic gold nanostructure,” ACS Nano 12, 7117–7126 (2018).
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S. Tan, Y. Dai, S. Zhang, L. Liu, J. Zhao, and H. Petek, “Coherent electron transfer at the Ag/graphite heterojunction interface,” Phys. Rev. Lett. 120, 126801 (2018).
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H. Lee, J. Lim, C. Lee, S. Back, K. An, J. W. Shin, R. Ryoo, Y. Jung, and J. Y. Park, “Boosting hot electron flux and catalytic activity at metal-oxide interfaces of PtCo bimetallic nanoparticles,” Nat. Commun. 9, 2335 (2018).
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T. Mohammad, T. Hossein, X. Zihao, L. Kyu-Tae, R. Sean, Y. Jiahao, A. Ali, L. Tianquan, and C. Wenshan, “Ultrafast control of phase and polarization of light expedited by hot electron transfer,” Nano Lett. 18, 5544–5551 (2018).
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Y. Liu, M. Jiang, Z. Zhang, B. Li, H. Zhao, C. Shan, and D. Shen, “Electrically excited hot-electron dominated fluorescent emitters using individual Ga-doped ZnO microwires via metal quasiparticle film decoration,” Nanoscale 10, 5678–5688 (2018).
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J. H. Park, Y. K. Dong, E. F. Schubert, J. Cho, and J. K. Kim, “Fundamental limitations of wide-bandgap semiconductors for light-emitting diodes,” ACS Energy Lett. 3, 655–662 (2018).
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J. Feng, C. Gao, and Y. Ying, “Nanoscale tracking plasmon-driven photocatalysis in individual nanojunctions by vibrational spectroscopy,” Nanoscale 10, 20492–20504 (2018).
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H. Wei, D. Pan, S. Zhang, Z. Li, Q. Li, N. Liu, W. Wang, and H. Xu, “Plasmon waveguiding in nanowires,” Chem. Rev. 118, 2882–2926 (2018).
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2017 (16)

M. Cohen, Y. Abulafia, R. Shavit, and Z. Zalevsky, “Secondary electron imaging of light at the nanoscale,” ACS Nano 11, 3274–3281 (2017).
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P. Zilio, M. Dipalo, F. Tantussi, G. C. Messina, and F. D. Angelis, “Hot electrons in water: injection and ponderomotive acceleration by means of plasmonic nanoelectrodes,” Light Sci. Appl. 6, e17002 (2017).
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S. Wang, J. Wang, W. Zhao, F. Giustiniano, L. Chu, I. Verzhbitskiy, Y. J. Zhou, and G. Eda, “Efficient carrier-to-exciton conversion in field emission tunnel diodes based on MIS-type van der Waals heterostack,” Nano Lett. 17, 5156–5162 (2017).
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S. A. K. Cushing, “Plasmonic hot carriers skip out in femtoseconds,” Nat. Photonics 11, 748–749 (2017).
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S. Tan, A. Argondizzo, J. Ren, L. Liu, Z. Jin, and H. Petek, “Plasmonic coupling at a metal/semiconductor interface,” Nat. Photonics 11, 806–812 (2017).
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S. Ganti, P. J. King, E. Arac, K. Dawson, M. J. Heikkil, J. H. Quilter, B. Murdoch, P. Cumpson, and A. O’Neill, “Voltage controlled hot carrier injection enables ohmic contacts using Au island metal films on Ge,” ACS Appl. Mater. Interfaces 9, 27357–27364 (2017).
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S. Tan, L. Liu, Y. Dai, J. Ren, J. Zhao, and H. Petek, “Ultrafast plasmon-enhanced hot electron generation at Ag nanocluster/graphite heterojunctions,” J. Am. Chem. Soc. 139, 6160–6168 (2017).
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M. Jiang, G. He, H. Chen, Z. Zhang, L. Zheng, C. Shan, D. Shen, and X. Fang, “Wavelength-tunable electroluminescent light sources from individual Ga-doped ZnO microwires,” Small 13, 1604034 (2017).
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B. Zhao, W. Fei, H. Chen, L. Zheng, L. Su, D. Zhao, and X. Fang, “An ultrahigh responsivity (9.7 mA·W–1) self-powered solar-blind photodetector based on individual ZnO-Ga2O3 heterostructures,” Adv. Funct. Mater. 27, 1700264 (2017).
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G. H. He, M. M. Jiang, L. Dong, Z. Zhang, and D. Shen, “Near-infrared light-emitting devices from individual heavily Ga-doped ZnO microwires,” J. Mater. Chem. C 5, 2542–2551 (2017).
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K. Hu, F. Teng, L. Zheng, P. Yu, Z. Zhang, H. Chen, and X. Fang, “Binary response Se/ZnO p-n heterojunction UV photodetector with high on/off ratio and fast speed,” Laser Photon. Rev. 11, 1600257 (2017).
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W. Zhang, M. Caldarola, B. Pradhan, and M. Orrit, “Gold nanorod enhanced fluorescence enables single-molecule electrochemistry of methylene blue,” Angew. Chem. 129, 3620–3623 (2017).
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Y. Liu, M. Jiang, G. He, S. Li, Z. Zhang, B. Li, H. Zhao, C. Shan, and D. Z. Shen, “Wavelength-tunable ultraviolet electroluminescence from Ga-doped ZnO microwires,” ACS Appl. Mater. Interfaces 9, 40743–40751 (2017).
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F. F. Qin, C. X. Xu, Q. X. Zhu, J. F. Lu, D. T. You, W. Xu, Z. Zhu, A. G. Manohari, and F. Chen, “Extra green light induced ZnO ultraviolet lasing enhancement assisted by Au surface plasmons,” Nanoscale 10, 623–627 (2017).
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S. P. Gurunarayanan, N. Verellen, V. S. Zharinov, F. James Shirley, V. V. Moshchalkov, M. Heyns, J. Van de Vondel, I. P. Radu, and P. Van Dorpe, “Electrically driven unidirectional optical nanoantennas,” Nano Lett. 17, 7433–7439 (2017).
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G. H. He, M. M. Jiang, Z. Zhang, B. H. Li, H. Zhao, C. X. Shan, and D. Shen, “Sb-doped ZnO microwires: emitting filament and homojunction light-emitting diodes,” J. Mater. Chem. C 5, 10938–10946 (2017).
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2016 (3)

W. T. Ruane, K. M. Johansen, K. D. Leedy, D. C. Look, W. H. Von, M. Grundmann, G. C. Farlow, and L. J. Brillson, “Defect segregation and optical emission in ZnO nano- and microwires,” Nanoscale 8, 7631–7637 (2016).
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G. Lozano, S. R. Rodriguez, M. A. Verschuuren, and J. G. Rivas, “Metallic nanostructures for efficient led lighting,” Light Sci. Appl. 5, e16080 (2016).
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X. Li, J. Zhu, and B. Wei, “Hybrid nanostructures of metal/two-dimensional nanomaterials for plasmon-enhanced applications,” Chem. Soc. Rev. 45, 3145–3187 (2016).
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2015 (6)

Y. D. Kim, H. Kim, Y. Cho, J. H. Ryoo, C.-H. Park, P. Kim, Y. S. Kim, S. Lee, Y. Li, S.-N. Park, Y. S. Yoo, D. Yoon, V. E. Dorgan, E. Pop, T. F. Heinz, J. Hone, S.-H. Chun, H. Cheong, S. W. Lee, M.-H. Bae, and Y. D. Park, “Bright visible light emission from graphene,” Nat. Nanotechnol. 10, 676–682 (2015).
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B. Zhao, F. Wang, H. Chen, Y. Wang, M. Jiang, X. Fang, and D. Zhao, “Solar-blind avalanche photodetector based on single ZnO-Ga2O3 core-shell microwire,” Nano Lett. 15, 3988–3993 (2015).
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M. Buret, A. V. Uskov, J. Dellinger, N. Cazier, M.-M. Mennemanteuil, J. Berthelot, I. V. Smetanin, I. E. Protsenko, G. Colas-des Francs, and A. Bouhelier, “Spontaneous hot-electron light emission from electron-fed optical antennas,” Nano Lett. 15, 5811–5818 (2015).
[Crossref]

A. M. Brown, R. Sundararaman, P. Narang, and H. A. Atwater, “Nonradiative plasmon decay and hot carrier dynamics: effects of phonons, surfaces, and geometry,” ACS Nano 10, 957–966 (2015).
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B. Y. Zheng, H. Zhao, A. Manjavacas, M. McClain, P. Nordlander, and N. J. Halas, “Distinguishing between plasmon-induced and photoexcited carriers in a device geometry,” Nat. Commun. 6, 7797 (2015).
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K. H. Shokri, J. H. Yun, Y. Paik, J. Kim, W. A. Anderson, and S. J. Kim, “Plasmon field effect transistor for plasmon to electric conversion and amplification,” Nano Lett. 16, 250–254 (2015).
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2014 (3)

R. Sundararaman, P. Narang, A. S. Jermyn, and H. A. Atwater, “Theoretical predictions for hot-carrier generation from surface plasmon decay,” Nat. Commun. 5, 5788 (2014).
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A. Pescaglini, A. Martin, D. Cammi, G. Juska, C. Ronning, E. Pelucchi, and D. Iacopino, “Hot-electron injection in Au nanorod-ZnO nanowire hybrid device for near-infrared photodetection,” Nano Lett. 14, 6202–6209 (2014).
[Crossref]

M. K. Seo, K. C. Huang, and M. L. Brongersma, “Electrically driven subwavelength optical nanocircuits,” Nat. Photonics 8, 244–249 (2014).
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2013 (4)

N. Han, F. Wang, J. J. Hou, S. P. Yip, H. Lin, F. Xiu, M. Fang, Z. Yang, X. Shi, G. Dong, T. F. Hung, and J. C. Ho, “Tunable electronic transport properties of metal-cluster-decorated III–V nanowire transistors,” Adv. Mater. 25, 4445–4451 (2013).
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P. Rai, N. Hartmann, J. Berthelot, J. Arocas, G. C. des Francs, A. Hartschuh, and A. Bouhelier, “Electrical excitation of surface plasmons by an individual carbon nanotube transistor,” Phys. Rev. Lett. 111, 026804 (2013).
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A. Sobhani, M. W. Knight, Y. Wang, B. Zheng, N. S. King, L. V. Brown, Z. Fang, P. Nordlander, and N. J. Halas, “Narrowband photodetection in the near-infrared with a plasmon-induced hot electron device,” Nat. Commun. 4, 1643 (2013).
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X. Liu, Q. Zhang, J. N. Yip, Q. Xiong, and T. C. Sum, “Wavelength tunable single nanowire lasers based on surface plasmon polariton enhanced Burstein–Moss effect,” Nano Lett. 13, 5336–5343 (2013).
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2012 (2)

Y. Fang, W.-S. Chang, B. Willingham, P. Swanglap, S. Dominguez-Medina, and S. Link, “Plasmon emission quantum yield of single gold nanorods as a function of aspect ratio,” ACS Nano 6, 7177–7184 (2012).
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M. Ding, D. Zhao, B. Yao, E. Shulin, Z. Guo, L. Zhang, and D. Shen, “The ultraviolet laser from individual ZnO microwire with quadrate cross section,” Opt. Express 20, 13657–13662 (2012).
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2011 (2)

B. Palash, B. Alexandre, and N. Lukas, “Electrical excitation of surface plasmons,” Phys. Rev. Lett. 106, 226802 (2011).
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J. Zhao, H. Sun, S. Dai, Y. Wang, and J. Zhu, “Electrical breakdown of nanowires,” Nano Lett. 11, 4647–4651 (2011).
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2010 (1)

Y. Nishijima, K. Ueno, Y. Yokota, K. Murakoshi, and H. Misawa, “Plasmon-assisted photocurrent generation from visible to near-infrared wavelength using a Au-nanorods/TiO2 electrode,” J. Phys. Chem. Lett. 1, 2031–2036 (2010).
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2009 (1)

W. Cai, R. Sainidou, J. Xu, A. Polman, and F. J. G. de Abajo, “Efficient generation of propagating plasmons by electron beams,” Nano Lett. 9, 1176–1181 (2009).
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2008 (2)

G. D. Yuan, W. J. Zhang, J. S. Jie, X. Fan, J. X. Tang, I. Shafiq, Z. Z. Ye, C. S. Lee, and S. T. Lee, “Tunable n-type conductivity and transport properties of Ga-doped ZnO nanowire arrays,” Adv. Mater. 20, 168–173 (2008).
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P. Pramod and K. G. Thomas, “Plasmon coupling in dimers of Au nanorods,” Adv. Mater. 20, 4300–4305 (2008).
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2002 (1)

F. Kim, J. H. Song, and P. Yang, “Photochemical synthesis of gold nanorods,” J. Am. Chem. Soc. 124, 14316–14317 (2002).
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1972 (1)

P. B. Johnson and R.-W. Christy, “Optical constants of the noble metals,” Phys. Rev. B 6, 4370–4379 (1972).
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Abulafia, Y.

M. Cohen, Y. Abulafia, R. Shavit, and Z. Zalevsky, “Secondary electron imaging of light at the nanoscale,” ACS Nano 11, 3274–3281 (2017).
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Alexandre, B.

B. Palash, B. Alexandre, and N. Lukas, “Electrical excitation of surface plasmons,” Phys. Rev. Lett. 106, 226802 (2011).
[Crossref]

Ali, A.

T. Mohammad, T. Hossein, X. Zihao, L. Kyu-Tae, R. Sean, Y. Jiahao, A. Ali, L. Tianquan, and C. Wenshan, “Ultrafast control of phase and polarization of light expedited by hot electron transfer,” Nano Lett. 18, 5544–5551 (2018).
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Almqvist, N.

C. De Melo, M. Jullien, Y. Battie, A. En Naciri, J. Ghanbaja, F. Montaigne, J. F. Pierson, F. Rigoni, N. Almqvist, A. Vomiero, S. Migot, F. Mucklich, and D. Horwat, “Tunable localized surface plasmon resonance and broadband visible photoresponse of Cu nanoparticles/ZnO surfaces,” ACS Appl. Mater. Interfaces 10, 40958–40965 (2018).
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An, K.

H. Lee, J. Lim, C. Lee, S. Back, K. An, J. W. Shin, R. Ryoo, Y. Jung, and J. Y. Park, “Boosting hot electron flux and catalytic activity at metal-oxide interfaces of PtCo bimetallic nanoparticles,” Nat. Commun. 9, 2335 (2018).
[Crossref]

Anderson, W. A.

K. H. Shokri, J. H. Yun, Y. Paik, J. Kim, W. A. Anderson, and S. J. Kim, “Plasmon field effect transistor for plasmon to electric conversion and amplification,” Nano Lett. 16, 250–254 (2015).
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Angelis, F. D.

P. Zilio, M. Dipalo, F. Tantussi, G. C. Messina, and F. D. Angelis, “Hot electrons in water: injection and ponderomotive acceleration by means of plasmonic nanoelectrodes,” Light Sci. Appl. 6, e17002 (2017).
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Arac, E.

S. Ganti, P. J. King, E. Arac, K. Dawson, M. J. Heikkil, J. H. Quilter, B. Murdoch, P. Cumpson, and A. O’Neill, “Voltage controlled hot carrier injection enables ohmic contacts using Au island metal films on Ge,” ACS Appl. Mater. Interfaces 9, 27357–27364 (2017).
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Argondizzo, A.

S. Tan, A. Argondizzo, J. Ren, L. Liu, Z. Jin, and H. Petek, “Plasmonic coupling at a metal/semiconductor interface,” Nat. Photonics 11, 806–812 (2017).
[Crossref]

Arocas, J.

P. Rai, N. Hartmann, J. Berthelot, J. Arocas, G. C. des Francs, A. Hartschuh, and A. Bouhelier, “Electrical excitation of surface plasmons by an individual carbon nanotube transistor,” Phys. Rev. Lett. 111, 026804 (2013).
[Crossref]

Atwater, H. A.

A. M. Brown, R. Sundararaman, P. Narang, and H. A. Atwater, “Nonradiative plasmon decay and hot carrier dynamics: effects of phonons, surfaces, and geometry,” ACS Nano 10, 957–966 (2015).
[Crossref]

R. Sundararaman, P. Narang, A. S. Jermyn, and H. A. Atwater, “Theoretical predictions for hot-carrier generation from surface plasmon decay,” Nat. Commun. 5, 5788 (2014).
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Back, S.

H. Lee, J. Lim, C. Lee, S. Back, K. An, J. W. Shin, R. Ryoo, Y. Jung, and J. Y. Park, “Boosting hot electron flux and catalytic activity at metal-oxide interfaces of PtCo bimetallic nanoparticles,” Nat. Commun. 9, 2335 (2018).
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Bae, M.-H.

Y. D. Kim, H. Kim, Y. Cho, J. H. Ryoo, C.-H. Park, P. Kim, Y. S. Kim, S. Lee, Y. Li, S.-N. Park, Y. S. Yoo, D. Yoon, V. E. Dorgan, E. Pop, T. F. Heinz, J. Hone, S.-H. Chun, H. Cheong, S. W. Lee, M.-H. Bae, and Y. D. Park, “Bright visible light emission from graphene,” Nat. Nanotechnol. 10, 676–682 (2015).
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Barbosa, E. C. M.

I. F. Teixeira, E. C. M. Barbosa, S. C. E. Tsang, and P. H. C. Camargo, “Carbon nitrides and metal nanoparticles: from controlled synthesis to design principles for improved photocatalysis,” Chem. Soc. Rev. 47, 7783–7817 (2018).
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Battie, Y.

C. De Melo, M. Jullien, Y. Battie, A. En Naciri, J. Ghanbaja, F. Montaigne, J. F. Pierson, F. Rigoni, N. Almqvist, A. Vomiero, S. Migot, F. Mucklich, and D. Horwat, “Tunable localized surface plasmon resonance and broadband visible photoresponse of Cu nanoparticles/ZnO surfaces,” ACS Appl. Mater. Interfaces 10, 40958–40965 (2018).
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Berger, P. R.

T. A. Growden, W. Zhang, E. R. Brown, D. F. Storm, D. J. Meyer, and P. R. Berger, “Near-UV electroluminescence in unipolar-doped, bipolar-tunneling GaN/AlN heterostructures,” Light. Sci. Appl. 7, 17150 (2018).
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Berthelot, J.

M. Buret, A. V. Uskov, J. Dellinger, N. Cazier, M.-M. Mennemanteuil, J. Berthelot, I. V. Smetanin, I. E. Protsenko, G. Colas-des Francs, and A. Bouhelier, “Spontaneous hot-electron light emission from electron-fed optical antennas,” Nano Lett. 15, 5811–5818 (2015).
[Crossref]

P. Rai, N. Hartmann, J. Berthelot, J. Arocas, G. C. des Francs, A. Hartschuh, and A. Bouhelier, “Electrical excitation of surface plasmons by an individual carbon nanotube transistor,” Phys. Rev. Lett. 111, 026804 (2013).
[Crossref]

Bouhelier, A.

M. Buret, A. V. Uskov, J. Dellinger, N. Cazier, M.-M. Mennemanteuil, J. Berthelot, I. V. Smetanin, I. E. Protsenko, G. Colas-des Francs, and A. Bouhelier, “Spontaneous hot-electron light emission from electron-fed optical antennas,” Nano Lett. 15, 5811–5818 (2015).
[Crossref]

P. Rai, N. Hartmann, J. Berthelot, J. Arocas, G. C. des Francs, A. Hartschuh, and A. Bouhelier, “Electrical excitation of surface plasmons by an individual carbon nanotube transistor,” Phys. Rev. Lett. 111, 026804 (2013).
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Brillson, L. J.

W. T. Ruane, K. M. Johansen, K. D. Leedy, D. C. Look, W. H. Von, M. Grundmann, G. C. Farlow, and L. J. Brillson, “Defect segregation and optical emission in ZnO nano- and microwires,” Nanoscale 8, 7631–7637 (2016).
[Crossref]

Brongersma, M. L.

M. K. Seo, K. C. Huang, and M. L. Brongersma, “Electrically driven subwavelength optical nanocircuits,” Nat. Photonics 8, 244–249 (2014).
[Crossref]

Brown, A. M.

A. M. Brown, R. Sundararaman, P. Narang, and H. A. Atwater, “Nonradiative plasmon decay and hot carrier dynamics: effects of phonons, surfaces, and geometry,” ACS Nano 10, 957–966 (2015).
[Crossref]

Brown, E. R.

T. A. Growden, W. Zhang, E. R. Brown, D. F. Storm, D. J. Meyer, and P. R. Berger, “Near-UV electroluminescence in unipolar-doped, bipolar-tunneling GaN/AlN heterostructures,” Light. Sci. Appl. 7, 17150 (2018).
[Crossref]

Brown, L. V.

A. Sobhani, M. W. Knight, Y. Wang, B. Zheng, N. S. King, L. V. Brown, Z. Fang, P. Nordlander, and N. J. Halas, “Narrowband photodetection in the near-infrared with a plasmon-induced hot electron device,” Nat. Commun. 4, 1643 (2013).
[Crossref]

Buret, M.

M. Buret, A. V. Uskov, J. Dellinger, N. Cazier, M.-M. Mennemanteuil, J. Berthelot, I. V. Smetanin, I. E. Protsenko, G. Colas-des Francs, and A. Bouhelier, “Spontaneous hot-electron light emission from electron-fed optical antennas,” Nano Lett. 15, 5811–5818 (2015).
[Crossref]

Cai, W.

W. Cai, R. Sainidou, J. Xu, A. Polman, and F. J. G. de Abajo, “Efficient generation of propagating plasmons by electron beams,” Nano Lett. 9, 1176–1181 (2009).
[Crossref]

Cai, Y. Y.

Y. Y. Cai, J. G. Liu, L. J. Tauzin, D. Huang, E. Sung, H. Zhang, A. Joplin, W. S. Chang, P. Nordlander, and S. Link, “Photoluminescence of gold nanorods: Purcell effect enhanced emission from hot carriers,” ACS Nano 12, 976–985 (2018).
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Caldarola, M.

W. Zhang, M. Caldarola, B. Pradhan, and M. Orrit, “Gold nanorod enhanced fluorescence enables single-molecule electrochemistry of methylene blue,” Angew. Chem. 129, 3620–3623 (2017).
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Camargo, P. H. C.

I. F. Teixeira, E. C. M. Barbosa, S. C. E. Tsang, and P. H. C. Camargo, “Carbon nitrides and metal nanoparticles: from controlled synthesis to design principles for improved photocatalysis,” Chem. Soc. Rev. 47, 7783–7817 (2018).
[Crossref]

Cammi, D.

A. Pescaglini, A. Martin, D. Cammi, G. Juska, C. Ronning, E. Pelucchi, and D. Iacopino, “Hot-electron injection in Au nanorod-ZnO nanowire hybrid device for near-infrared photodetection,” Nano Lett. 14, 6202–6209 (2014).
[Crossref]

Cazier, N.

M. Buret, A. V. Uskov, J. Dellinger, N. Cazier, M.-M. Mennemanteuil, J. Berthelot, I. V. Smetanin, I. E. Protsenko, G. Colas-des Francs, and A. Bouhelier, “Spontaneous hot-electron light emission from electron-fed optical antennas,” Nano Lett. 15, 5811–5818 (2015).
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Chang, W. S.

Y. Y. Cai, J. G. Liu, L. J. Tauzin, D. Huang, E. Sung, H. Zhang, A. Joplin, W. S. Chang, P. Nordlander, and S. Link, “Photoluminescence of gold nanorods: Purcell effect enhanced emission from hot carriers,” ACS Nano 12, 976–985 (2018).
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Chang, W.-S.

Y. Fang, W.-S. Chang, B. Willingham, P. Swanglap, S. Dominguez-Medina, and S. Link, “Plasmon emission quantum yield of single gold nanorods as a function of aspect ratio,” ACS Nano 6, 7177–7184 (2012).
[Crossref]

Chen, C. J.

S. K. Cushing, C. J. Chen, C. L. Dong, X. T. Kong, A. O. Govorov, R. S. Liu, and N. Wu, “Tunable nonthermal distribution of hot electrons in a semiconductor injected from a plasmonic gold nanostructure,” ACS Nano 12, 7117–7126 (2018).
[Crossref]

Chen, D.

Chen, F.

F. F. Qin, C. X. Xu, Q. X. Zhu, J. F. Lu, D. T. You, W. Xu, Z. Zhu, A. G. Manohari, and F. Chen, “Extra green light induced ZnO ultraviolet lasing enhancement assisted by Au surface plasmons,” Nanoscale 10, 623–627 (2017).
[Crossref]

Chen, H.

B. Zhao, W. Fei, H. Chen, L. Zheng, L. Su, D. Zhao, and X. Fang, “An ultrahigh responsivity (9.7 mA·W–1) self-powered solar-blind photodetector based on individual ZnO-Ga2O3 heterostructures,” Adv. Funct. Mater. 27, 1700264 (2017).
[Crossref]

M. Jiang, G. He, H. Chen, Z. Zhang, L. Zheng, C. Shan, D. Shen, and X. Fang, “Wavelength-tunable electroluminescent light sources from individual Ga-doped ZnO microwires,” Small 13, 1604034 (2017).
[Crossref]

K. Hu, F. Teng, L. Zheng, P. Yu, Z. Zhang, H. Chen, and X. Fang, “Binary response Se/ZnO p-n heterojunction UV photodetector with high on/off ratio and fast speed,” Laser Photon. Rev. 11, 1600257 (2017).
[Crossref]

B. Zhao, F. Wang, H. Chen, Y. Wang, M. Jiang, X. Fang, and D. Zhao, “Solar-blind avalanche photodetector based on single ZnO-Ga2O3 core-shell microwire,” Nano Lett. 15, 3988–3993 (2015).
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Chen, H.-M.

C.-C. Hou, H.-M. Chen, J.-C. Zhang, N. Zhuo, Y.-Q. Huang, R. A. Hogg, D. T. Childs, J.-Q. Ning, Z.-G. Wang, F.-Q. Liu, and Z.-Y. Zhang, “Near-infrared and mid-infrared semiconductor broadband light emitters,” Light Sci. Appl. 7, 17170 (2018).
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Cheng, L.

Cheong, H.

Y. D. Kim, H. Kim, Y. Cho, J. H. Ryoo, C.-H. Park, P. Kim, Y. S. Kim, S. Lee, Y. Li, S.-N. Park, Y. S. Yoo, D. Yoon, V. E. Dorgan, E. Pop, T. F. Heinz, J. Hone, S.-H. Chun, H. Cheong, S. W. Lee, M.-H. Bae, and Y. D. Park, “Bright visible light emission from graphene,” Nat. Nanotechnol. 10, 676–682 (2015).
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Childs, D. T.

C.-C. Hou, H.-M. Chen, J.-C. Zhang, N. Zhuo, Y.-Q. Huang, R. A. Hogg, D. T. Childs, J.-Q. Ning, Z.-G. Wang, F.-Q. Liu, and Z.-Y. Zhang, “Near-infrared and mid-infrared semiconductor broadband light emitters,” Light Sci. Appl. 7, 17170 (2018).
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Figures (7)

Fig. 1.
Fig. 1. EL emission characteristics from single AuNRs@ZnO:Ga MW-based incandescent-type light source (the extinction peak of Au-nanorod, 695 nm). (a) The extinction spectrum of Au nanorods, with corresponding TEM image of the Au nanorods demonstrated in the inset. (b) SEM image of single AuNRs@ZnO:Ga MW. (c) Amplified SEM image of Au nanorods deposited on the MW. (d) IV characteristics of single ZnO:Ga MW prepared via Au nanorods decoration. (e) EL emission spectra from single ZnO:Ga MW-based fluorescent emitter. (f) EL emission spectra from single AuNRs@ZnO:Ga MW-based incandescent-type light source. (g) Optical microscopic image of the light emitting from electrically biased single ZnO:Ga MW-based fluorescent emitter (scale bar, 200 μm). (h) Optical microscopic image of the light emitting from electrically biased single AuNRs@ZnO:Ga MW-based incandescent-type light source (scale bar, 200 μm).
Fig. 2.
Fig. 2. (a) Optical photograph of the synthesized ZnO:Ga MWs. (b) SEM image of single ZnO:Ga MW, with perfect quadrilateral cross section displayed in the inset (scale bar, 12 μm). (c) SEM image of ZnO:Ga MW prepared with Au nanorods decoration (the spin-coating number, ×1). (d) TEM images of the Au nanorods with controlled aspect ratio. (e) The extinction spectra of Au nanorods with controlled aspect ratio. (f) PL emissions from ZnO:Ga MW prepared via Au nanorods decoration, with the controlled aspect ratios. (g) IV behaviors of single ZnO:Ga MW prepared with Au nanorods decoration (corresponding extinction peak centered at 695 nm), with the spin-coating number ranging from 0 to 6.
Fig. 3.
Fig. 3. Photoconductive behavior of single AuNRs@ZnO:Ga MW [Au nanorod in Fig. 2(d) panel II, the extinction peak, 695 nm]. (a) Schematic diagram of hot carrier generation mechanisms in plasmonic Au nanorods, and then injected into ZnO:Ga MW channel under light illumination. (b) The IV characteristics of single ZnO:Ga MW prepared with Au nanorods decoration under dark, and illumination with the excitation lasing wavelengths at 405 nm, 532 nm, and 685 nm, respectively, with the laser power density denoted as 5.0  mW/cm2. (c) The It characteristics with on/off switching under light illumination, with the lasing wavelengths at 405 nm, 532 nm, and 685 nm, respectively. (d) UV-vis absorption spectra of the as-synthesized ZnO:Ga MWs prepared with and without Au nanorods deposition. (e) The comparison of TRPL decays from single bare ZnO:Ga MW, and Au nanorods decorated ZnO:Ga MW. (f) Diagrammatic drawing of the physical process involving (i) photoexcitation induced electrons and (ii) plasmons induced generation, injection, or tunneling procedure of hot electrons towards the interface between Au-ZnO:Ga under light illumination.
Fig. 4.
Fig. 4. Electrical field intensity |E/E0|2 distribution of isolated Au-nanorods, with the electromagnetic wave propagating along (a) the x direction of the xy plane (horizontal), (b) the y direction of the xy plane (vertical), and (c) the x direction of the xz plane (horizontal). In the simulation process, Au-nanorods with the length (50 nm) and diameter (20 nm) were adopted, accompanied with the resonant wavelength denoted as λ=695  nm, the refractive index of ZnO:Ga denoted as nZnO:Ga=2.45, and the refractive index of environmental medium air nair=1.0.
Fig. 5.
Fig. 5. (a) Schematic illustration of the modulation of Au-nanorod plasmons on the incandescent-type lighting features of single ZnO:Ga MW-based fluorescent light source. (b) Normalized intensities of the EL spectrum from single bare ZnO:Ga MW-based fluorescent light source, the EL spectrum from single AuNRs@ZnO:Ga MW-based fluorescent light source, and the extinction spectrum of the deposited Au nanorods. (c) Micrographs of bright visible light emitting from an electrically driven single AuNRs@ZnO:Ga MW-based incandescent-type light source in the dark field and bright field (scale bar, 200 μm). (d) Optical microscopic images of bright visible light emitting from electrically driven single ZnO:Ga MW prepared with partial Au nanorods decoration (scale bar, 300 μm).
Fig. 6.
Fig. 6. Schematic diagram of the working principle of bright visible light emitting from electrically biased single AuNRs@ZnO:Ga MW-based incandescent-type light source.
Fig. 7.
Fig. 7. Wavelength-tunable emissions from single AuNRs@ZnO:Ga MW-based incandescent-type light source: (a) IV characteristics of single ZnO:Ga MW via Au nanorods decoration (the extinction peak, 605 nm); (b) EL emission from single bare ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered at 527 nm; (c) EL emission from single AuNRs@ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered at 601 nm. (d) IV characteristics of single ZnO:Ga MW prepared via Au nanorods decoration (the extinction peak, 783 nm); (e) EL emission from single bare ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered at 518 nm; (f) EL emission from the single AuNRs@ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered around 780 nm. (g) IV characteristics of single ZnO:Ga MW via Au nanorods decoration (the extinction peak, 855 nm); (h) EL emission from the single bare ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered at 513 nm; (i) EL emission from the single AuNRs@ZnO:Ga MW-based incandescent-type light source, with the emission wavelength centered around 905 nm.

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