Abstract

Magneto-optical (MO) composites with excellent Faraday rotation (FR) response were fabricated using iron platinum (FePt) nanoparticles (NPs) and polystyrene-block-poly (2-vinyl pyridine) (PS-b-P2VP) block copolymers (BCPs). Gallic acid functionalized FePt NPs with average core diameters (dcore) of 1.9, 4.9, 5.7 and 9.3 nm have been selectively incorporated into a P2VP domain through hydrogen bonding interactions. The use of copolymer templates to selectively arrange the magnetic NPs guaranteed high MO performance with little trade-off in terms of scattering loss, providing a simple strategy to prepare functional materials for MO applications. As a result, Verdet constants of a 10 wt % loaded 4.9 nm FePt NP composite reached absolute magnitudes as high as ~-6 × 104 °/T-m at 845 nm, as determined by FR measurements at room temperature. At the same time, the MO figure-of-merit was as large as −25 °/T in these composites, indicating both excellent MO performance and transparency. The dependence of the nanocomposite FR properties on particle diameter, loading (from 0.1 wt % to 10 wt %) and composite nanostructure were systematically investigated at four infrared wavelengths (845, 980, 1310 and 1550 nm).

© 2017 Optical Society of America

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2016 (1)

D. P. Song, C. Li, W. Li, and J. J. Watkins, “Block copolymer nanocomposites with high refractive index contrast for one-step photonics,” ACS Nano 10(1), 1216–1223 (2016).
[Crossref] [PubMed]

2015 (5)

D. P. Song, C. Li, C. S. Nicholas, X. Lu, J.-H. Lee, and J. J. Watkins, “Thermally tunable metallodielectric photonic crystals from the self-assembly of brush block copolymers and gold nanoparticles,” Adv. Opt. Mater. 3(9), 1169–1175 (2015).
[Crossref]

D. P. Song, Y. Lin, Y. Gai, N. S. Colella, C. Li, X. H. Liu, S. Gido, and J. J. Watkins, “Controlled supramolecular self-assembly of large nanoparticles in amphiphilic brush block Copolymers,” J. Am. Chem. Soc. 137(11), 3771–3774 (2015).
[Crossref] [PubMed]

D. P. Song, C. Li, N. S. Colella, W. Xie, S. Li, X. Lu, S. Gido, J. H. Lee, and J. J. Watkins, “Large-volume self-organization of polymer/nanoparticle hybrids with millimeter-scale grain sizes using brush block copolymers,” J. Am. Chem. Soc. 137(39), 12510–12513 (2015).
[Crossref] [PubMed]

R. García, M. Ramírez-Del-Solar, J. M. González-Leal, E. Blanco, and M. Domínguez, “Improving Magnetooptical Faraday Effect of Maghemite/silica Nanocomposites,” Mater. Chem. Phys. 154, 1–9 (2015).
[Crossref]

B. J. H. Stadler and T. Mizumoto, “Integrated magneto-optical materials and isolators: a review,” IEEE Photonics J. 6, 0600215 (2015).

2014 (5)

P. Zu, C. C. Chan, G. W. Koh, W. S. Lew, Y. Jin, H. F. Liew, W. C. Wong, and X. Dong, “Enhancement of the sensitivity of magneto-optical fiber sensor by magnifying the birefringence of magnetic fluid film with loyt-sagnac interferometer,” Sens. Actuators B Chem. 191, 19–23 (2014).
[Crossref]

M. Moocarme, J. L. Domínguez-Juárez, and L. T. Vuong, “Ultralow-intensity magneto-optical and mechanical effects in metal nanocolloids,” Nano Lett. 14(3), 1178–1183 (2014).
[Crossref] [PubMed]

A. I. Savchuk, I. D. Stolyarchuk, V. V. Makoviy, and O. A. Savchuk, “Magneto-optical Faraday rotation of semiconductor nanoparticles embedded in dielectric matrices,” Appl. Opt. 53(10), B22–B26 (2014).
[Crossref] [PubMed]

L. Yao, Y. Lin, and J. J. Watkins, “Ultrahigh loading of nanoparticles into ordered block copolymer composites,” Macromolecules 47(5), 1844–1849 (2014).
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X. Wang, R. D. Tilley, and J. J. Watkins, “Simple ligand exchange reactions enabling excellent dispersibility and stability of magnetic nanoparticles in polar organic, aromatic, and protic solvents,” Langmuir 30(6), 1514–1521 (2014).
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2013 (7)

G. Armelles, A. Cebollada, A. Garcia-Martin, and M. U. Gonzalez, “Magnetoplasmonics: magnetoplasmonics: combining magnetic and plasmonic functionalities,” Adv. Opt. Mater. 1(1), 10–35 (2013).
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H. Cui, M. Wang, W. Ren, Y. Liu, and Y. Zhao, “Highly Transparent Silica Monoliths Embedded with High Concentration Oxide Nanoparticles,” J. Sol-Gel Sci. Technol. 66(3), 512–517 (2013).
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J. Kao, K. Thorkelsson, P. Bai, B. J. Rancatore, and T. Xu, “Toward functional nanocomposites: taking the best of nanoparticles, polymers, and small molecules,” Chem. Soc. Rev. 42(7), 2654–2678 (2013).
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S. Taccola, F. Greco, A. Zucca, C. Innocenti, C. de Julián Fernández, G. Campo, C. Sangregorio, B. Mazzolai, and V. Mattoli, “Characterization of free-standing PEDOT:PSS/iron oxide nanoparticle composite thin films and application as conformable humidity sensors,” ACS Appl. Mater. Interfaces 5(13), 6324–6332 (2013).
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V. I. Belotelov, L. E. Kreilkamp, I. A. Akimov, A. N. Kalish, D. A. Bykov, S. Kasture, V. J. Yallapragada, A. Venu Gopal, A. M. Grishin, S. I. Khartsev, M. Nur-E-Alam, M. Vasiliev, L. L. Doskolovich, D. R. Yakovlev, K. Alameh, A. K. Zvezdin, and M. Bayer, “Plasmon-mediated magneto-optical transparency,” Nat. Commun. 4, 1–7 (2013).

R. Shimano, G. Yumoto, J. Y. Yoo, R. Matsunaga, S. Tanabe, H. Hibino, T. Morimoto, and H. Aoki, “Quantum Faraday and Kerr rotations in graphene,” Nat. Commun. 4, 1841 (2013).
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H. Majeed, A. Shaheen, and M. S. Anwar, “Complete stokes polarimetry of magneto-optical faraday effect in a terbium gallium garnet crystal at cryogenic temperatures,” Opt. Express 21(21), 25148–25158 (2013).
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2012 (7)

R. V. Mikhaylovskiy, E. Hendry, and V. V. Kruglyak, “Ultrafast Inverse Faraday Effect in a Paramagnetic Terbium Gallium Garnet Crystal,” Phys. Rev. B 86(10), 100405 (2012).
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A. Lopez-Santiago, H. R. Grant, P. Gangopadhyay, R. Voorakaranam, R. A. Norwood, and N. Peyghambarian, “Cobalt ferrite nanoparticles polymer composites based all-optical magnetometer,” Opt. Mater. Express 2(7), 978 (2012).
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R. M. Silva, H. Martins, I. Nascimento, J. M. Baptista, A. L. Ribeiro, J. L. Santos, P. Jorge, and O. Frazão, “Optical current sensors for high power systems: a review,” Appl. Sci. 2(4), 602–628 (2012).
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S. G. Jang, A. Khan, C. J. Hawker, and E. J. Kramer, “morphology evolution of PS-B-P2VP diblock copolymers via supramolecular assembly of hydroxylated gold nanoparticles,” Macromolecules 45(3), 1553–1561 (2012).
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Q. Wei, Y. Lin, E. R. Anderson, A. L. Briseno, S. P. Gido, and J. J. Watkins, “Additive-driven assembly of block copolymer-nanoparticle hybrid materials for solution processable floating gate memory,” ACS Nano 6(2), 1188–1194 (2012).
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M. J. Fernée, C. Sinito, Y. Louyer, C. Potzner, T.-L. Nguyen, P. Mulvaney, P. Tamarat, and B. Lounis, “Magneto-optical properties of trions in non-blinking charged nanocrystals reveal an acoustic phonon bottleneck,” Nat. Commun. 3, 1287 (2012).
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Q. Dong, G. Li, C. L. Ho, M. Faisal, C. W. Leung, P. W. T. Pong, K. Liu, B. Z. Tang, I. Manners, and W. Y. Wong, “A polyferroplatinyne precursor for the rapid fabrication of L1(0) -FePt-type bit patterned media by nanoimprint lithography,” Adv. Mater. 24(8), 1034–1040 (2012).
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2011 (10)

T. Bublat and D. Goll, “Large-area hard magnetic L10-FePt nanopatterns by nanoimprint lithography,” Nanotechnology 22(31), 315301 (2011).
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L. Wang, C. Clavero, Z. Huba, K. J. Carroll, E. E. Carpenter, D. Gu, and R. A. Lukaszew, “Plasmonics and enhanced magneto-optics in core-shell co-ag nanoparticles,” Nano Lett. 11(3), 1237–1240 (2011).
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Y. Lin, V. K. Daga, E. R. Anderson, S. P. Gido, and J. J. Watkins, “Nanoparticle-driven assembly of block copolymers: a simple route to ordered hybrid materials,” J. Am. Chem. Soc. 133(17), 6513–6516 (2011).
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S. G. Jang, E. J. Kramer, and C. J. Hawker, “Controlled supramolecular assembly of micelle-like gold nanoparticles in PS-b-P2VP diblock copolymers via hydrogen bonding,” J. Am. Chem. Soc. 133(42), 16986–16996 (2011).
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J. M. Caicedo, O. Pascu, M. López-García, V. Canalejas, A. Blanco, C. López, J. Fontcuberta, A. Roig, and G. Herranz, “Magnetophotonic response of three-dimensional opals,” ACS Nano 5(4), 2957–2963 (2011).
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I. Crassee, J. Levallois, A. L. Walter, M. Ostler, A. Bostwick, E. Rotenberg, T. Seyller, D. van der Marel, and A. B. Kuzmenko, “Giant Faraday rotation in single- and multilayer graphene,” Nat. Phys. 7(1), 48–51 (2011).
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V. I. Belotelov, I. A. Akimov, M. Pohl, V. A. Kotov, S. Kasture, A. S. Vengurlekar, A. V. Gopal, D. R. Yakovlev, A. K. Zvezdin, and M. Bayer, “Enhanced magneto-optical effects in magnetoplasmonic crystals,” Nat. Nanotechnol. 6(6), 370–376 (2011).
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V. Bonanni, S. Bonetti, T. Pakizeh, Z. Pirzadeh, J. Chen, J. Nogués, P. Vavassori, R. Hillenbrand, J. Åkerman, and A. Dmitriev, “Designer magnetoplasmonics with nickel nanoferromagnets,” Nano Lett. 11(12), 5333–5338 (2011).
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M. Veis, E. Lišková, R. Antoš, Š. Višňovský, N. Kumar, D. S. Misra, N. Venkataramani, S. Prasad, and R. Krishnan, “Polar and longitudinal magneto-optical spectroscopy of bismuth substituted yttrium iron garnet films grown by pulsed laser deposition,” Thin Solid Films 519(22), 8041–8046 (2011).
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M. A. Schmidt, L. Wondraczek, H. W. Lee, N. Granzow, N. Da, and P. St J Russell, “Complex Faraday rotation in microstructured magneto-optical fiber waveguides,” Adv. Mater. 23(22-23), 2681–2688 (2011).
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2010 (1)

E. A. Jackson and M. A. Hillmyer, “Nanoporous membranes derived from block copolymers: from drug delivery to water filtration,” ACS Nano 4(7), 3548–3553 (2010).
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2009 (7)

J. Bang, U. Jeong, Y. Ryu, T. P. Russell, and C. J. Hawker, “Block copolymer nanolithography: translation of molecular level control to nanoscale patterns,” Adv. Mater. 21(47), 4769–4792 (2009).
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A. Lopez-Santiago, P. Gangopadhyay, J. Thomas, R. A. Norwood, A. Persoons, and N. Peyghambarian, “Faraday rotation in magnetite-polymethylmethacrylate core-shell nanocomposites with high optical quality,” Appl. Phys. Lett. 95(14), 143302 (2009).
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P. K. Jain, Y. Xiao, R. Walsworth, and A. E. Cohen, “Surface plasmon resonance enhanced rotation enhancement in gold-coated iron oxide nanocrystals,” Nano Lett. 9, 1644 (2009).
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A. Lopez-Satiago, P. Gangopadhyay, J. Thomas, R. A. Norwood, A. Persoons, and N. Peyghambarian, “Faraday rotation in magnetite-polymethylmethacrylate core shell nanocomposites with high optical quality,” Appl. Phys. Lett. 95(14), 143302 (2009).
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Y. Zhao, K. Thorkelsson, A. J. Mastroianni, T. Schilling, J. M. Luther, B. J. Rancatore, K. Matsunaga, H. Jinnai, Y. Wu, D. Poulsen, J. M. J. Fréchet, A. P. Alivisatos, and T. Xu, “Small-molecule-directed nanoparticle assembly towards stimuli-responsive nanocomposites,” Nat. Mater. 8(12), 979–985 (2009).
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R. Lewicki, J. H. Doty, R. F. Curl, F. K. Tittel, and G. Wysocki, “Ultrasensitive detection of nitric oxide at 5.33 microm by using external cavity quantum cascade laser-based Faraday rotation spectroscopy,” Proc. Natl. Acad. Sci. U.S.A. 106(31), 12587–12592 (2009).
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P. Siddons, N. C. Bell, Y. Cai, C. S. Adams, and I. G. A. Hughes, “Gigahertz-bandwidth atomic probe based on the slow-light Faraday effect,” Nat. Photonics 3(4), 225–229 (2009).
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2008 (4)

M. Domínguez, D. Ortega, J. S. Garitaonandía, R. Litrán, C. Barrera-Solano, E. Blanco, and M. Ramírez-del-Solar, “Magneto-optic Faraday effect in maghemite nanoparticles/silica matrix nanocomposites prepared by the sol-gel method,” J. Magn. Magn. Mater. 320(20), e725–e729 (2008).
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K. Hayashi, R. Fujikawa, W. Sakamoto, M. Inoue, and T. Yogo, “Synthesis of Highly Transparent Lithium Ferrite Nanoparticle/polymer Hybrid Self-Standing Films Exhibiting Faraday Rotation in the Visible Region,” J. Phys. Chem. C 112(37), 14255–14261 (2008).
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C. Tang, E. M. Lennon, G. H. Fredrickson, E. J. Kramer, and C. J. Hawker, “Evolution of block copolymer lithography to highly ordered square arrays,” Science 322(5900), 429–432 (2008).
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P. Gangopadhyay, R. Voorakaranam, A. Lopez-Santiago, S. Foerier, J. Thomas, R. A. Norwood, A. Persoons, and N. Peyghambarian, “Faraday rotation measurements on thin films of regioregular alkyl-substituted polythiophene derivatives,” J. Phys. Chem. C 112(21), 8032–8037 (2008).
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2007 (2)

R. Gerritsma, S. Whitlock, T. Fernholz, H. Schlatter, J. Luigjes, J. U. Thiele, J. B. Goedkoop, and R. J. C. Spreeuw, “Lattice of microtraps for ultracold atoms based on patterned magnetic films,” Phys. Rev. A 76(3), 033408 (2007).
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V. Nandwana, K. E. Elkins, N. Poudyal, G. S. Chaubey, K. Yano, and J. P. Liu, “Size and shape control of monodisperse FePt nanoparticles,” J. Phys. Chem. C 111(11), 4185–4189 (2007).
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2006 (4)

S. Sun, “Recent advances in chemical synthesis, self-assembly, and applications of FePt nanoparticles,” Adv. Mater. 18(4), 393–403 (2006).
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J. Y. Cheng, C. A. Ross, H. I. Smith, and E. L. Thomas, “Templated self-assembly of block copolymers: top-down helps bottom-up,” Adv. Mater. 18(19), 2505–2521 (2006).
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A. C. Balazs, T. Emrick, and T. P. Russell, “Nanoparticle polymer composites: where two small worlds meet,” Science 314(5802), 1107–1110 (2006).
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R. Bahuguna, M. Mina, J. W. Tioh, and R. J. Weber, “Magneto-Optic-based fiber switch for optical communications,” IEEE Trans. Magn. 42(10), 3099–3101 (2006).
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2005 (3)

S. Y. Sung, X. Qi, and B. J. H. Stadler, “Integrating yttrium iron garnet onto nongarnet substrates with faster deposition rates and high reliability,” Appl. Phys. Lett. 87(12), 1–3 (2005).
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M. R. Bockstaller, R. A. Mickiewicz, and E. L. Thomas, “Block copolymer nanocomposites: perspectives for tailored functional materials,” Adv. Mater. 17(11), 1331–1349 (2005).
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A. V. Ruzette and L. Leibler, “Block copolymers in tomorrow’s plastics,” Nat. Mater. 4(1), 19–31 (2005).
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2004 (3)

Q. Guo, X. Teng, and H. Yang, “Fabrication of magnetic FePt patterns from langmuir-blodgett films of platinum-iron oxide core-shell nanoparticles,” Adv. Mater. 16(15), 1337–1341 (2004).
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T. Y. Kim, Y. Yamazaki, and T. Hirano, “Magneto-optical properties of Bi-YIG nanoparticle with polymethacrylate matrix materials,” Phys. Status Solidi Basic Res. 241(7), 1601–1604 (2004).
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M. Laulajainen, P. Paturi, J. Raittila, H. Huhtinen, A. B. Abrahamsen, N. H. Andersen, and R. Laiho, “BixY3-xFe5O12 Thin films prepared by laser ablation for magneto-optical imaging of superconducting thin films,” J. Magn. Magn. Mater. 279(2-3), 218–223 (2004).
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2003 (1)

M. Zayat, F. Del Monte, M. Del Puerto Morales, G. Rosa, H. Guerrero, C. J. Serna, and D. Levy, “Highly transparent γ-Fe2O3/Vycor-glass magnetic nanocomposites exhibiting Faraday rotation,” Adv. Mater. 15(21), 1809–1812 (2003).
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2002 (2)

E. M. Moreno, M. Zayat, M. P. Morales, C. J. Serna, A. Roig, and D. Levy, “Preparation of Narrow Size Distribution Superparamagnetic,” Langmuir 18(12), 4972–4978 (2002).
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J. Y. Lee, R. B. Thompson, D. Jasnow, and A. C. Balazs, “Entropically driven formation of hierarchically ordered nanocomposites,” Phys. Rev. Lett. 89(15), 155503 (2002).
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2001 (5)

W. A. Lopes and H. M. Jaeger, “Hierarchical self-assembly of metal nanostructures on diblock copolymer scaffolds,” Nature 414(6865), 735–738 (2001).
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H. A. Klok and S. Lecommandoux, “Supramolecular materials via block copolymer self-assembly,” Adv. Mater. 13(16), 1217–1229 (2001).
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Z. H. Zhou, J. M. Xue, H. S. O. Chan, and J. Wang, “Transparent magnetic composites of ZnFe2O4 nanoparticles in silica,” J. Appl. Phys. 90(8), 4169–4174 (2001).
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A. B. Villaverde, D. A. Donatti, and D. G. Bozinis, “Terbium gallium garnet Verdet constant measurements with pulsed magnetic field,” J. Phys. C Solid State Phys. 11(12), L495–L498 (2001).
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P. Tartaj, T. Gonzalez-carreo, and C. J. Serna, “Single-step nanoengineering of silica coated maghemite hollow spheres with tunable magnetic properties,” Adv. Mater. 13(21), 1620–1624 (2001).
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2000 (3)

T. Yogo, T. Nakamura, W. Sakamoto, and S. Hirano, “Synthesis of transparent magnetic particle/organic hybrid film using iron-organics,” J. Mater. Res. 15(10), 2114–2120 (2000).
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T. Thurn-Albrecht, J. Schotter, G. A. Kästle, N. Emley, T. Shibauchi, L. Krusin-Elbaum, K. Guarini, C. T. Black, M. T. Tuominen, and T. P. Russell, “Ultrahigh-density nanowire arrays grown in self-assembled diblock copolymer templates,” Science 290(5499), 2126–2129 (2000).
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S. Sun, C. B. Murray, D. Weller, L. Folks, and A. Moser, “Monodisperse FePt nanoparticles and ferromagnetic fept nanocrystal superlattices,” Science 287(5460), 1989–1992 (2000).
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1997 (1)

L. L. Beecroft and C. K. Ober, “Nanocomposite materials for optical applications,” Chem. Mater. 9(6), 1302–1317 (1997).
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1992 (1)

R. F. Ziolo, E. P. Giannelis, B. A. Weinstein, M. P. O’horo, B. N. Ganguly, V. Mehrotra, M. W. Russell, and D. R. Huffman, “Matrix-mediated synthesis of nanocrystalline ggr-Fe2O3: a new optically transparent magnetic material,” Science 257(5067), 219–223 (1992).
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1990 (1)

V. Doormann, J. P. Krumme, and H. Lenz, “Optical and magneto-optical tensor spectra of bismuth-substituted yttrium-iron-garnet films,” J. Appl. Phys. 68(7), 3544–3553 (1990).
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1989 (1)

P. Hansen, C. Clausen, G. Much, M. Rosenkranz, and K. Witter, “Magnetic and Magneto-optical properties of rare-earth transition-metal alloys containing Gd, Tb, Fe, Co,” J. Appl. Phys. 66(2), 756–767 (1989).
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1975 (1)

G. Scott, D. Lacklison, H. Ralph, and J. Page, “Magnetic circular dichroism and Faraday rotation spectra of Y3Fe5O12,” Phys. Rev. B 12(7), 2562–2571 (1975).
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1973 (1)

D. E. Lacklison, G. B. Scott, H. I. Ralph, and J. L. Page, “Garnets with high magnetooptic figures of merit in the visible region,” IEEE Trans. Magn. 9(3), 457–460 (1973).
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1972 (1)

J. C. Suits, “Faraday and Kerr effects in magnetic compounds,” IEEE Trans. Magn. 8(1), 95–105 (1972).
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1964 (1)

N. Borrelli, “Faraday rotation in glasses,” J. Chem. Phys. 41(11), 3289–3293 (1964).
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Abrahamsen, A. B.

M. Laulajainen, P. Paturi, J. Raittila, H. Huhtinen, A. B. Abrahamsen, N. H. Andersen, and R. Laiho, “BixY3-xFe5O12 Thin films prepared by laser ablation for magneto-optical imaging of superconducting thin films,” J. Magn. Magn. Mater. 279(2-3), 218–223 (2004).
[Crossref]

Adams, C. S.

P. Siddons, N. C. Bell, Y. Cai, C. S. Adams, and I. G. A. Hughes, “Gigahertz-bandwidth atomic probe based on the slow-light Faraday effect,” Nat. Photonics 3(4), 225–229 (2009).
[Crossref]

Åkerman, J.

V. Bonanni, S. Bonetti, T. Pakizeh, Z. Pirzadeh, J. Chen, J. Nogués, P. Vavassori, R. Hillenbrand, J. Åkerman, and A. Dmitriev, “Designer magnetoplasmonics with nickel nanoferromagnets,” Nano Lett. 11(12), 5333–5338 (2011).
[Crossref] [PubMed]

Akimov, I. A.

V. I. Belotelov, L. E. Kreilkamp, I. A. Akimov, A. N. Kalish, D. A. Bykov, S. Kasture, V. J. Yallapragada, A. Venu Gopal, A. M. Grishin, S. I. Khartsev, M. Nur-E-Alam, M. Vasiliev, L. L. Doskolovich, D. R. Yakovlev, K. Alameh, A. K. Zvezdin, and M. Bayer, “Plasmon-mediated magneto-optical transparency,” Nat. Commun. 4, 1–7 (2013).

V. I. Belotelov, I. A. Akimov, M. Pohl, V. A. Kotov, S. Kasture, A. S. Vengurlekar, A. V. Gopal, D. R. Yakovlev, A. K. Zvezdin, and M. Bayer, “Enhanced magneto-optical effects in magnetoplasmonic crystals,” Nat. Nanotechnol. 6(6), 370–376 (2011).
[Crossref] [PubMed]

Alameh, K.

V. I. Belotelov, L. E. Kreilkamp, I. A. Akimov, A. N. Kalish, D. A. Bykov, S. Kasture, V. J. Yallapragada, A. Venu Gopal, A. M. Grishin, S. I. Khartsev, M. Nur-E-Alam, M. Vasiliev, L. L. Doskolovich, D. R. Yakovlev, K. Alameh, A. K. Zvezdin, and M. Bayer, “Plasmon-mediated magneto-optical transparency,” Nat. Commun. 4, 1–7 (2013).

Alivisatos, A. P.

Y. Zhao, K. Thorkelsson, A. J. Mastroianni, T. Schilling, J. M. Luther, B. J. Rancatore, K. Matsunaga, H. Jinnai, Y. Wu, D. Poulsen, J. M. J. Fréchet, A. P. Alivisatos, and T. Xu, “Small-molecule-directed nanoparticle assembly towards stimuli-responsive nanocomposites,” Nat. Mater. 8(12), 979–985 (2009).
[Crossref] [PubMed]

Andersen, N. H.

M. Laulajainen, P. Paturi, J. Raittila, H. Huhtinen, A. B. Abrahamsen, N. H. Andersen, and R. Laiho, “BixY3-xFe5O12 Thin films prepared by laser ablation for magneto-optical imaging of superconducting thin films,” J. Magn. Magn. Mater. 279(2-3), 218–223 (2004).
[Crossref]

Anderson, E. R.

Q. Wei, Y. Lin, E. R. Anderson, A. L. Briseno, S. P. Gido, and J. J. Watkins, “Additive-driven assembly of block copolymer-nanoparticle hybrid materials for solution processable floating gate memory,” ACS Nano 6(2), 1188–1194 (2012).
[Crossref] [PubMed]

Y. Lin, V. K. Daga, E. R. Anderson, S. P. Gido, and J. J. Watkins, “Nanoparticle-driven assembly of block copolymers: a simple route to ordered hybrid materials,” J. Am. Chem. Soc. 133(17), 6513–6516 (2011).
[Crossref] [PubMed]

Antoš, R.

M. Veis, E. Lišková, R. Antoš, Š. Višňovský, N. Kumar, D. S. Misra, N. Venkataramani, S. Prasad, and R. Krishnan, “Polar and longitudinal magneto-optical spectroscopy of bismuth substituted yttrium iron garnet films grown by pulsed laser deposition,” Thin Solid Films 519(22), 8041–8046 (2011).
[Crossref]

Anwar, M. S.

Aoki, H.

R. Shimano, G. Yumoto, J. Y. Yoo, R. Matsunaga, S. Tanabe, H. Hibino, T. Morimoto, and H. Aoki, “Quantum Faraday and Kerr rotations in graphene,” Nat. Commun. 4, 1841 (2013).
[Crossref] [PubMed]

Armelles, G.

G. Armelles, A. Cebollada, A. Garcia-Martin, and M. U. Gonzalez, “Magnetoplasmonics: magnetoplasmonics: combining magnetic and plasmonic functionalities,” Adv. Opt. Mater. 1(1), 10–35 (2013).
[Crossref]

Bahuguna, R.

R. Bahuguna, M. Mina, J. W. Tioh, and R. J. Weber, “Magneto-Optic-based fiber switch for optical communications,” IEEE Trans. Magn. 42(10), 3099–3101 (2006).
[Crossref]

Bai, P.

J. Kao, K. Thorkelsson, P. Bai, B. J. Rancatore, and T. Xu, “Toward functional nanocomposites: taking the best of nanoparticles, polymers, and small molecules,” Chem. Soc. Rev. 42(7), 2654–2678 (2013).
[Crossref] [PubMed]

Balazs, A. C.

A. C. Balazs, T. Emrick, and T. P. Russell, “Nanoparticle polymer composites: where two small worlds meet,” Science 314(5802), 1107–1110 (2006).
[Crossref] [PubMed]

J. Y. Lee, R. B. Thompson, D. Jasnow, and A. C. Balazs, “Entropically driven formation of hierarchically ordered nanocomposites,” Phys. Rev. Lett. 89(15), 155503 (2002).
[Crossref] [PubMed]

Bang, J.

J. Bang, U. Jeong, Y. Ryu, T. P. Russell, and C. J. Hawker, “Block copolymer nanolithography: translation of molecular level control to nanoscale patterns,” Adv. Mater. 21(47), 4769–4792 (2009).
[Crossref] [PubMed]

Baptista, J. M.

R. M. Silva, H. Martins, I. Nascimento, J. M. Baptista, A. L. Ribeiro, J. L. Santos, P. Jorge, and O. Frazão, “Optical current sensors for high power systems: a review,” Appl. Sci. 2(4), 602–628 (2012).
[Crossref]

Barrera-Solano, C.

M. Domínguez, D. Ortega, J. S. Garitaonandía, R. Litrán, C. Barrera-Solano, E. Blanco, and M. Ramírez-del-Solar, “Magneto-optic Faraday effect in maghemite nanoparticles/silica matrix nanocomposites prepared by the sol-gel method,” J. Magn. Magn. Mater. 320(20), e725–e729 (2008).
[Crossref]

Bayer, M.

V. I. Belotelov, L. E. Kreilkamp, I. A. Akimov, A. N. Kalish, D. A. Bykov, S. Kasture, V. J. Yallapragada, A. Venu Gopal, A. M. Grishin, S. I. Khartsev, M. Nur-E-Alam, M. Vasiliev, L. L. Doskolovich, D. R. Yakovlev, K. Alameh, A. K. Zvezdin, and M. Bayer, “Plasmon-mediated magneto-optical transparency,” Nat. Commun. 4, 1–7 (2013).

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Figures (7)

Fig. 1
Fig. 1 (a) Surface modification of FePt NPs using gallic acid (GA) as a hydrogen bonding donor followed by selective NP dispersion in the P2VP domain within a symmetric PS-b-P2VP BCP template. (b) Illustration of Faraday rotation, the rotation of polarization angle depends on the Verdet constant (V) of medium, applied magnetic field (B) and path length of the light (L).
Fig. 2
Fig. 2 Schematic drawing of the homodyne Faraday rotation measurement system with a sinusoidal magnetic field; the purple line represents the second pass through the sample; GT is a Glan Thomson polarizer and NPBS is a non-polarizing beam splitter. Black arrows along the optical path denote polarization states.
Fig. 3
Fig. 3 TEM images of GA capped FePt NPs and corresponding histograms with average core diameter dcore (a) 1.9 nm, (b) 4.9 nm, (c) 5.7 nm and (d) 9.3nm.
Fig. 4
Fig. 4 Crystal structure of size controlled FePt particles: (a) XRD spectrum of dcore ~ 5.7 nm and 9.3 nm FePt NPs powder, fcc characteristic peaks agree with previous results; (b) dcore ~ 9.3 nm and (c) dcore ~ 5.7 nm are electron diffraction images, the halo pattern corresponds to the XRD spectrum calibrated with a gold standard sample.
Fig. 5
Fig. 5 (a) Room temperature SAXS profiles of neat PS (102 kg/mol)-b-P2VP (97 kg/mol) with 1.9 nm, 4.9 nm, 5.7 nm and 9.3 nm FePt NPs at 2.5 wt % loading; primary peaks indicate strong phase separation of NP/BCP blends; representative TEM images of 10 wt % loading of (b) 1.9 nm NPs and (c) 9.3 nm NPs in block copolymer. The P2VP domain was lightly stained with iodine - particles show selective distribution through favorable H-bonding interactions.
Fig. 6
Fig. 6 Hysteresis loops of 2.5 wt %1.9 nm, 5.5 nm, X = 3-4 nm, Y = 6-7 nm and 9.3nm FePt NPs in PS (102 kg/mol)-b-P2VP (97 kg/mol) composite. The magnetization falls back to zero in absence of the applied magnetic field for all sizes of particles. The saturation value of magnetization showed clear size dependency.
Fig. 7
Fig. 7 The MO figure of merit (FOM) plotted vs. number density for particle sizes (a) 1.9 nm, (b) 4.8 nm, (c) 5.7 nm and (d) 9.3 nm at the four wavelengths studied. The FOM was calculated from Verdet constant and film absorption coefficient, which was determined by UV-vis spectroscopy (see SI Table S3-S6). Particle number density was calculated based on NP size and TGA data.

Tables (3)

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Table 1 FePt NPs core weight and volume fraction (fNP,,%) in the nanocomposites

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Table 2 Verdet constants (V) for the glass substrate

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Table 3 Verdet constants (V) of FePt NP/BCP composite films (104 °/T⋅m) a

Equations (3)

Equations on this page are rendered with MathJax. Learn more.

I t h =k I o sin( 2n θ 0 sin( ωt ) ),      I t v =k I 0 sin( π 2 2n θ 0 sin( ωt ) )
θ 0 = 180 π | I ac h (ω) rms I ac v (ω) rms | 2n g i ( I dc h + I dc v )
FOM= V(°/Tm) α( m 1 )

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