The ir and Raman spectroscopic studies of metal complexes with nitrogen-containing ligands have been reviewed. A special emphasis has been placed on the stretching and bending fundamentals of the metal–ligand bond. The following ligands are included in the discussion: nitrosyl, nitro, nitrite, nitride, azido, molecular nitrogen, hydrazine, isocyanate, isothiocyanate, isoselenocyanate, pyridine, and ethylenediamine.

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