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  • Frontiers in Optics 2007/Laser Science XXIII/Organic Materials and Devices for Displays and Energy Conversion
  • OSA Technical Digest (CD) (Optica Publishing Group, 2007),
  • paper FThA2
  • https://doi.org/10.1364/FIO.2007.FThA2

Search for Pure Vibrational Dephasing of Electronically Excited Dye Molecules in Solution

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Abstract

10 fs pulses compressed with Brewster-angled chirped mirrors are used to measure the vibronic wavepacket motion in a perylene dye. The coherence lifetime of 1.0 - 1.5 ps indicates that vibrational relaxation and pure dephasing contribute equally.

© 2007 Optical Society of America

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